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State-to-State Dynamical Research in the F+H2 Reaction System

ST: STATE TO STATE DYNAMICAL RSRCH F+H2 REACTION SYSTEM

Chemistry

Mathematics & Science

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B2B GT

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B2B & B2C

This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of F+H2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg 'tagging' time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the F+H2 reaction, a precise measurement of the differential cross section in the F+HD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F*(2P1/2) in the F+D2 reaction, and exploits the breakdown of BOA in the low collision energy.

POST SECONDARY FOUR YEAR

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Duration

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Front Cover.
Half Title Page.
Other Front Matter.
Title Page.
Copyright Page.
Other Front Matter.
Supervisor&#x0027;s Foreword.
Acknowledgments.
Contents.
1: Introduction.
2: Hydrogen Atom Rydberg Tagging Time-of-Flight Crossed Molecular Beam Apparatus.
3: Dynamical Resonances in F + H2.
4: The Non-Adiabatic Effects in F(2P) + D2 &#x2192; DF + D.
Postscript.

State-to-State Dynamical Research in the F+H2 Reaction System.css-1p8rvzy{position:absolute;padding-left:8px;}

State-to-State Dynamical Research in the F+H2 Reaction System